ANTIMONY HALIDES

Antimony trichloride SbCl3

SbCl3 for Sb2Te3, Ge2Sb2Te5 by ALD

     Antimony trichloride SbCl3 (combined with Te(SiEt3)2) has been applied as antimony precursor for the CVD growth of Sb2Te3 films at temperature as low as 60°C, as well as for the  ALD growth of the phase change material GST (germanium antimony telluride, Ge2Sb2Te5)  (with GeCl2·C4H8O2 as germanium source). The byproduct in both ALD processes was Et3SiCl, and about 78% (36%) of it was released during the SbCl3 (GeCl2·C4H8O2) pulse. It was concluded that Te(SiEt3) surface groups serve as reactive sites for the metal precursors, cf. −OH surface groups in the oxide ALD processes that use water as the oxygen source. The mechanism of the SbCl3-(Et3Si)2Te reaction during GST deposition changed in the way that during the SbCl3 pulse only ~50% of the Et3SiCl byproduct was released. When the SbCl3-(Et3Si)2Te process was executed on Al2O3 and Au substrates surfaces, similar effect was observed as well.  [[i]]

 [i] Kjell Knapas, Timo Hatanpää, Mikko Ritala and Markku Leskelä, Chem. Mater., 2010, 22 (4), pp 1386–1391

Antimony pentachloride SbCl5

SbCl5 for Sb-Ge-S glass films by CVD

Antimony pentachloride SbCl5 was used as a precursor for the deposition of Sb-Ge-S glass films [560]

SbCl5 for GeSb films by CVD

    Antimony pentachloride SbCl5 , in combination with GeCl4 as Ge source, and 6%H2/Ar (50-200sccm) has been used as antimony precursor for the CVD growth of GeSb films [[i],[ii]]

[i] C.C. Huang, B.Gholipour, J.Y. Ou,  K.Knight, D.W. Hewak, Electron. Lett., 2011,, Vol.47 , Iss.4, p. 288 - 289

[ii] DW Hewak, CC Huang, B Gholipour, F Al-Saab… - epcos.org, «  Thermally Stable, Low Current Consuming Gallium and Germanium Chalcogenides for Consumer and Automotive Memory Applications », http://www.epcos.org/library/papers/pdf_2011/Oral-Papers/S3-04.pdf

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